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The Belgian montes (public pawnshops) continued to charge 15% on pawns up to the French Revolution (422) While no specific rates are quoted here, it is certain that far higher rates were charged and collected on usurious personal loans and risk loans of a commercial and political character Sweden during the seventeenth and eighteenth centuries made an interesting contribution to the history of European interest rates, even though the data are confined to rates established by law The Bank of Sweden was founded in 1656 This was shortly after the abdication of Queen Christina and on the eve of the absolute rule and military adventures of her successors, Charles X, XI, and XII The bank in 1661 started the first official issue of bank notes in Europe thirty-three years before the founding of the Bank of England However, the experiment was not pressed, and note issue was discontinued in 1664.

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Some early polymerizations reported as Ziegler Natta polymerizations were conventional free-radical, cationic, or anionic polymerizations proceeding with low stereoselectivity. Some Ziegler Natta initiators contain components that are capable of initiating conventional ionic polymerizations of certain monomers, such as anionic polymerization of methacrylates by alkyllithium and cationic polymerization of vinyl ethers by TiCl4 . Most Ziegler Natta components participate in a complex set of reactions involving alkylation and reduction of the transition-metal component by the group I III component as shown below for TiCl4 AlR3 :

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TiCl 4 + AlR3 TiCl 4 + AlR2Cl TiCl 3R + AlR3 TiCl 3R TiCl 3 + AlR3 R TiCl 3R + AlR2Cl TiCl 3R + AlRCl2 TiCl 2R2 + AlRCl2 TiCl 3 + R TiCl 2R + AlR2Cl

8-28 8-29 8-30 8-31 8-32 8-33

In the laws governing the Bank of Sweden the interest rate paid on deposits was fixed at 6% in 1668, while the rates charged for bank loans were fixed at 8% for large loans, 81 4% for smaller loans, and 105 32% for small loans (423) These were roughly comparable to English commercial loan rates at the time, but were far above the very low 3 4% Dutch rates The Dutch example impressed the Estates of Sweden, which expressed the desire that their bank would eventually lower its loaning rates at least to 6% The bank in fact lowered the rate that it paid on deposits to 41 2% in 1669 in compliance with a royal decree, and in 1687 it lowered its maximum loan rate to 6%.

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Radicals produced in Eq. 8-31 are capable of initiating radical polymerizations with some monomers, for example, vinyl chloride. The mechanism for the stereoselective polymerization of a-ole ns and other nonpolar alkenes is a p-complexation of monomer and transition metal (utilizing the latter s d-orbitals) followed by a four-center anionic coordination insertion process in which monomer is inserted into a metal carbon bond as described in Fig. 8-10. Support for the initial p-complexation has come from ESR, NMR, and IR studies [Bur eld, 1984]. The insertion reaction has both cationic and anionic features. There is a concerted nucleophilic attack by the incipient carbanion polymer chain end on the a-carbon of the double bond together with an electrophilic attack by the cationic counterion on the alkene p-electrons. The anionic character of the polymerization is consistent with the polymerization rate decreasing in the order ethylene > propene > 1-butene [Bier, 1961; Boor, 1967]. The reverse order is expected for a polymerization involving the conversion of a monomer into the corresponding carbocation. For addition of a carbanion to the monomers, attack occurs at the a-carbon to form the less substituted (and more stable) carbanion. Further, a-substituents sterically hinder the approach of a carbanion and/or counterion with the result that reactivity decreases with increasing substituent size. Evidence for the anionic nature of propagation also comes from studies in which labeled methanol is used to terminate chain growth. The terminated polymer is radioactive when CH3 O3 H is used, while termination by 14 CH3 OH yields a nonradioactive polymer [Bur eld and Savariar, 1979; Zakharov et al., 1977]. Additional veri cation comes from experiments with 14 CO and 14 CO2 [Mejzlik and Lesna, 1977]. 8-4c Primary versus Secondary Insertion; Regioselectivity

The insertion reaction shown in Fig. 8-10 is primary insertion (or 1,2-addition) the unsubstituted end of the double bond carries the partial negative charge and is attached to the counterion G. The other possibility is second insertion (or 2,1-addition) where the substituted end of the double bond becomes attached to G. The two modes of insertion are described by

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In 1700 the bank raised its deposit rate from 41 2 to 5%, but in 1701 it was again lowered by decree to 41 2% Apparently the decline in interest rates which during the first half of the eighteenth century spread from Holland to England and even to France eventually found reflection in Sweden This was after the spectacular military success of Charles XII of Sweden in his war against Peter the Great of Russia, after his final defeat in 1709 1714, and after constitutional government was re-established in Sweden, 1718 1720 In 1741 the rate for bank loans on precious metals was reduced from 6 to 41 2%, while.

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javascript convert pdf to tiff

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